Transition between Heavy-Fermion-Strange-Metal and Quantum Spin Liquid in a 4d-Electron Trimer Lattice. Journal Article uri icon

Overview

abstract

  • We present experimental evidence that a heavy Fermi surface consisting of itinerant, charge-neutral spinons underpins both heavy-fermion-strange-metal (without f electrons) and quantum-spin-liquid states in the 4d-electron trimer lattice, Ba_{4}Nb_{1-x}Ru_{3+x}O_{12}(-x-<0.20). These two exotic states both exhibit an extraordinarily large entropy, a linear heat capacity extending into the milli-Kelvin regime, a linear thermal conductivity at low temperatures, and separation of charges and spins. Furthermore, the insulating spin liquid is a much better thermal conductor than the heavy-fermion-strange-metal that separately is observed to strongly violate the Wiedemann-Franz law. We propose that at the heart of this 4d system is a universal, heavy spinon Fermi surface that provides a unified framework for explaining the exotic phenomena observed throughout the entire series. The control of such exotic ground states provided by variable Nb concentration offers a new paradigm for studies of correlated quantum matter.

publication date

  • May 31, 2024

has restriction

  • green

Date in CU Experts

  • June 12, 2024 2:40 AM

Full Author List

  • Zhao H; Zhang Y; Schlottmann P; Nandkishore R; DeLong LE; Cao G

author count

  • 6

Other Profiles

Electronic International Standard Serial Number (EISSN)

  • 1079-7114

Additional Document Info

start page

  • 226503

volume

  • 132

issue

  • 22